要红昌-郑州大学化学学院，平原实验室（郑州大学）

要红昌

作者：时间：2021-01-21 点击数：

111

要红昌，南京大学理学博士，香港中文大学访问学者。现任郑州大学化学学院教授，博士生/硕士导师。研究方向为可见光催化材料的设计合成和性能研究，以及气敏材料的制备及其在呼气分析、环境监测等领域的研究。主持和参与国家自然科学基金、河南省科技厅基金、河南省教育厅基金和郑州市科技局项目多项。近年来，以通讯作者或第一作者在Appl. Catal. B: Environm., ACS Appl. Mater. Interfaces, J. Power Sources, Sensors and Actuators B, J. CO₂Utilization, J. Hazard. Mater., Chem. Commun.等刊物上发表SCI论文50余篇。

联系方式:

邮箱:yaohongchang@zzu.edu.cn;hchyao111@163.com

主要研究方向：

1.光催化材料的制备及性能研究

环境污染和能源危机是当今世界面临的共同难题。利用太阳能分解水制氢、利用太阳能降解污染物以及利用太阳能把二氧化碳还原为有机化合物，为解决上述问题提供了有效途径。课题组通过金属离子掺杂、表面敏化、贵金属沉积以及半导体复合等方法设计合成新型的光催化剂，从而优化调控催化剂的光催化效率，实现污染物矿化、分解水制氢以及二氧化碳还原。相关研究成果已发表在Appl. Catal. B: Environm.,ACS Appl. Mater. Interf.,J. Hazard. Mater.,Catal. Comm.等期刊上。

2.半导体气敏材料的制备及其性能研究

气体传感器在环境监测、污染监控、煤矿安全、食品检测以及呼气分析等领域发挥着日益重要的作用。金属氧化物半导体气体传感器因灵敏度高、稳定性好、结构简单、价格便宜等特点而受到广泛关注。但半导体气敏材料存在着选择性差等缺点,限制了气体传感器在特定领域的发展和应用。课题组针对这些问题，根据半导体材料对不同气体的气敏机理，通过掺杂、纳米组装、功能化等技术的综合运用，从而达到对特定气体的选择性检测。相关研究成果已发表在ACS Appl. Mater. Interf.,Sens. Actuator B，IEEE Sensors J.等期刊上。

主持项目：

① 国家自然科学基金项目面上项目(No. 21471133)

多层有序介孔氧化钨薄膜的可控构筑及对痕量丙酮的气敏选择性研究

2015/1 – 2018/12 已结题主持

② 河南省高等学校重点科研项目(No. 20A150041)

三维有序大孔氧化钨气敏材料的构筑及检测呼气中痕量丙酮的应用研究

2020/1 – 2021/12 在研主持

③ 河南省教育厅科学技术研究重点项目(No.14A150001)

纳米碳掺杂WO₃的制备及其对痕量丙酮的选择性检测

2015/1 – 2018/12 已结题主持

④ 郑州市科技局项目(No.141PQYJS562)

纳米碳掺杂WO₃气敏材料的制备及其对呼气中痕量丙酮的选择性检测

2015/1 – 2018/12 已结题主持

代表性论文：

[1] Y.-K. Lv, Y.-Y. Li, R.-H. Zhou, Y.-P. Pan,H.-C. Yao^*, Z.-J. Li.Doped graphene quantum dots-decorated three-dimensionalordered macroporous In₂O₃for NO₂sensing at low temperatures.ACS Appl. Mater. Interfaces2020, 12, 34245−34253.

[2] R.-H. Zhou, Z.-H. Wei, Y.-Y. Li, Z.-J. Li,H.-C. Yao*. Construction of visible light–responsive Z-scheme CdS/BiOI photocatalyst with enhanced photocatalytic CO₂reduction activity.J. Mater. Res.2019, 34, 3907-3917.

[3] Y.-Y. Li, Z.-H. Wei, J.-B. Fan, Z.-J. Li*,H.-C. Yao*. Photocatalytic CO₂reduction activity of Z-scheme CdS/CdWO₄catalysts constructed by surface charge directed selective deposition of CdS.Appl. Surf. Sci.2019, 483, 442–452.

[4] L.-D. Zhao, Q. Zhang, J.-B. Fan, L.-Q. Yin, P.-W. Qi,H.-C. Yao*, Z.-J. Li*. Improvement of the photoelectrochemical performance of vertically aligned WO₃nanosheet array film with a disordered surface layer by electroreduction.J. Solid State Electrochem.2019, 23, 1621–1630.

[5] M.-D. Wang, Y.-Y. Li, B.-H. Yao, K. Zhai, Z.-J. Li,H.-C. Yao*. Synthesis of three-dimensionally ordered macro/mesoporous C-doped WO₃materials: Effffect of template sizes on gas sensing properties.Sensors & Actuators B2019, 288, 656–666.

[6] Y.-K. Lv, B.-H. Yao, Z.-Q. Liu, S. Liang, Q.-C. Liu*, K. Zhai*, Z.-J. Li,H.-C. Yao*. Hierarchical Au-loaded WO₃hollow microspheres with high sensitive and selective properties to toluene and xylene.IEEE Sensors J.2019, 19, 5413-5420.

[7] Q.-Z. Huang, Z.-J. Tao, L.-Q. Ye,H.-C. Yao*, Z.g-J. Li*. Mn_0.2Cd_0.8S nanowires modified by CoP₃nanoparticles for highly efficient photocatalytic H₂evolution under visible light irradiation.Appl. Catal. B: Environm.2018, 237, 689-698.

[8] Z.-H. Wei, Y.-F. Wang, Y.-Y. Li, L. Zhang,H.-C. Yao*, Z.-J. Li*. Enhanced photocatalytic CO₂reduction activity of Z-scheme CdS/BiVO₄nanocomposite with thinner BiVO₄nanosheets.J. CO₂Utilization2018, 28, 15-25.

[9] J.-Y. Shen, M.-D. Wang, Y.-F. Wang, J.-Y. Hu, Y. Zhu*, Y. X. Zhang*, Z.-J. Li,H.-C. Yao*. Iron and carbon codoped WO₃with hierarchical walnut-like microstructure for highly sensitive and selective acetone sensor.Sensors and Actuators B2018, 256, 27-37.

[10] Q.-Z. Huang, J.-C. Wang, L.-Q. Ye, Q. Zhang,H.-C. Yao*, Z.-J. Li*. A novel p–n heterojunction Mn_0.25Cd_0.75S/Co₃O₄for highly efficient photocatalytic H₂evolution under visible light irradiation.J. Taiwan Inst. Chem. E.2017, 80, 570–577.

[11] Q.-Z. Huang, Y. Xiong, Q. Zhang,H.-C. Yao*, Z.-J. Li*. Noble metal-free MoS₂modified Mn_0.25Cd_0.75S for highly efficient visible-light driven photocatalytic H₂.Appl. Catal. B: Environ.2017, 209, 514–522.

[12] Q.-Z. Huang, J.-C. Wang, P.-P. Wang,H.-C. Yao*, Z.-J. Li*. In-situ growth of mesoporous Nb₂O₅microspheres on g-C₃N₄nanosheets for enhanced photocatalytic H₂evolution under visible light irradiation.Int. J. Hydrogen Energy2017, 42, 6683-6694.

[13]J.-Y. Shen, L. Zhang, J. Ren, J.-C. Wang,H.-C. Yao*, Z.-J. Li*. Highly enhanced acetone sensing performance of porous C-doped WO₃hollow spheres by carbon spheres as templates.Sensors and Actuators B2017, 239, 597–607.

[14]J.-C. Wang,H.-C. Yao*,Z.-Y. Fan, L. Zhang, J.-S. Wang, S.-Q. Zang and Z.-J. Li*. Indirect Z-Scheme BiOI/g-C₃N₄Photocatalysts with Enhanced Photoreduction CO₂Activity under Visible Light Irradiation.ACS Appl. Mater. Interfaces,2016, 8, 3765-3775.

[15]J.-C. Wang, J. Ren,H.-C. Yao*, L. Zhang, J.-S. Wang, S.-Q. Zang, L.-F. Han, Z.-J. Li*. Synergistic Photocatalysis of Cr(VI) Reduction and 4-Chlorophenol Degradation over Hydroxylatedrmalpha-Fe₂O₃under Visible Light Irradiation.J. Hazard. Mater.2016, 311,11-19.

[16] X.-B. Wang, H.-Q. Zheng, H. Rao,H.-C. Yao*, Y.-T. Fan*, H.-W. Hou. Synthesis of a new iron–sulfur cluster compound and its photocatalytic H₂evolution activity through visible light irradiation.Appl. Organomet. Chem.2016, 30, 638-644.

[17]J.-C. Wang, L. Zhang, W.-X. Fang, J. Ren, Y.-Y. Li,H.-C. Yao*, J.-S. Wang, Z.-J. Li*. Enhanced Photoreduction CO₂Activity over Direct Z‑Scheme α‑Fe₂O₃/Cu₂O Heterostructures under Visible Light Irradiation.ACS Appl. Mater. Interfaces2015, 7, 8631−8639.

[18] T. Xiao, X.-Y. Wang, Z.-H. Zhao, L. Li, J.-S. Wang,H.-C. Yao*, Z.-J. Li.Highly sensitive and selective acetone sensor based on C-doped WO₃for potential diagnosis of diabetes mellitus.Sensors andActuator B2014, 199, 210-219.